A Hardy-like proof of quantum contextuality is a compelling way to see the conflict between quantum theory and noncontextual hidden variables (NCHVs), as the latter predict that a particular probability must be zero, while quantum theory predicts a nonzero value. For the existing Hardy-like proofs, the success probability tends to 1/2 when the number of measurement settings n goes to infinity. It means the conflict between the existing Hardy-like proof and NCHV theory is weak, which is not conducive to experimental observation. Here we advance the study of a stronger Hardy-like proof of quantum contextuality, whose success probability is always higher than the previous ones generated from a certain n-cycle graph. Furthermore, the success probability tends to 1 when n goes to infinity. We perform the experimental test of the Hardy-like proof in the simplest case of n=7 by using a four-dimensional quantum system encoded in the polarization and orbital angular momentum of single photons. The experimental result agrees with the theoretical prediction within experimental errors. In addition, by starting from our Hardy-like proof, one can establish the stronger noncontextuality inequality, for which the quantum-classical ratio is higher with the same n, which provides a new method to construct some optimal noncontextuality inequalities. Our results offer a way for optimizing and enriching exclusivity graphs, helping to explore more abundant quantum properties.

Optical orbital angular momentum (OAM) is a special property of photons and has evoked research onto the light–matter interaction in both classical and quantum regimes. In classical optics, OAM is related to an optical vortex with a helical phase structure. In quantum optics, photons with a twisted or helical phase structure will carry a quantized OAM. To our knowledge, however, so far, no experiment has demonstrated the fundamental property of the OAM at the single-photon level. In this Letter, we have demonstrated the average photon trajectories of twisted photons in a double-slit interference. We have experimentally captured the double-slit interference process of twisted photons by a time-gated intensified charge-coupled device camera, which is trigged by a heralded detection. Our work provides new perspectives for understanding the micro-behaviors of twisted particles and enables new applications in imaging and sensing.